期刊
CHEMISTRY OF MATERIALS
卷 28, 期 7, 页码 2441-2448出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.chemmater.6b00836
关键词
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资金
- Army Research Office - Young Investigator Program [W911NF-15-1-0610]
- U.S. Department of Energy-Basic Energy Sciences [DE-SC0014902]
- Department of Energy (DOE), Office of Science, Basic Energy Science (BES) [DE-SC0010307]
- Energy Frontier Research Center at Temple University - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012575]
- Targeted Research Grant from Temple University Office of the Vice Provost for Research
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38]
- U.S. Department of Energy (DOE) [DE-SC0014902, DE-SC0010307] Funding Source: U.S. Department of Energy (DOE)
Supramolecular assembly utilizing noncovalent interaction to construct ordered molecular charge-transfer solids has led to significant advancement and breakthrough in energy-efficient molecular electronics, memories and solar cells. However, to exploit the coupling across these different energy regimes, the method that is capable of manipulating charge-spinlattice interactions is indispensable. Here, by rational chemical design of the supramolecular assembled charge-transfer networks, opto-ferroic properties can be coupled, in which a collective electron transfer and ordering strongly influence the dipole and spin orders, as well as their coupling. The supramolecular charge-transfer crystal presented here opens up a new route for the development of multifunctional organics that can lead to significant advancement in molecular ferronics.
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