4.8 Article

Universal High-Energy Photoelectron Emission from Nanoclusters Beyond the Atomic Limit

期刊

PHYSICAL REVIEW LETTERS
卷 124, 期 17, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.124.173201

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资金

  1. Air Force Office of Scientific Research under MURI Grant [FA9550-16-1-0013]
  2. National Science Foundation [PHY-1605042]
  3. Ohio Supercomputer Center [PAS0207]

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Rescattering by electrons on classical trajectories is central to understand photoelectron and high-harmonic emission from isolated atoms or molecules in intense laser pulses. By controlling the cluster size and the quiver amplitude of electrons, we demonstrate how rescattering influences the energy distribution of photoelectrons emitted from noble gas nanoclusters. Our experiments reveal a universal dependence of photoelectron energy distributions on the cluster size when scaled by the field driven electron excursion, establishing a unified rescattering picture for extended systems with the known atomic dynamics as the limit of zero extension. The result is supported by molecular dynamics calculations and rationalized with a one-dimensional classical model.

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