期刊
CHEMICAL SOCIETY REVIEWS
卷 45, 期 15, 页码 4391-4436出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cs00873e
关键词
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资金
- Natural Sciences and Engineering Research Council of Canada (NSERC)
- Canada Research Chairs Program
- Ontario Research Chairs Program
CO2 is an ideal trigger for switchable or stimuli-responsive materials because it is benign, inexpensive, green, abundant, and does not accumulate in the system. Many different CO2-responsive materials including polymers, latexes, solvents, solutes, gels, surfactants, and catalysts have been prepared. This review focuses on the preparation, self-assembly, and functional applications of CO2-responsive polymers. Detailed discussion is provided on the synthesis of CO2-responsive polymers, in particular using reversible deactivation radical polymerization (RDRP), formerly known as controlled/living radical polymerization (CLRP), a powerful technique for the preparation of well-defined (co)polymers with precise control over molecular weight distribution, chain-end functional groups, and polymer architectural design. Self-assembly in aqueous dispersed media is highlighted as well as emerging potential applications.
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