期刊
ORGANIC LETTERS
卷 22, 期 17, 页码 6698-6702出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c01381
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资金
- Bill & Melinda Gates Foundation
A four-step synthesis of the dimeric pyrrol-imidazole alkaloid sceptrin is reported. The brevity of the route is based on a simple solution developed for selective assembly of the cyclobutane core of the natural product. The photochemical intermolecular [2 + 2] dimerization of a useful hymenidin surrogate enables direct entry to this enigmatic class of biologically active marine secondary metabolites.
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