期刊
CHEMICAL RECORD
卷 16, 期 6, 页码 2674-2686出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/tcr.201600055
关键词
asymmetric catalysis; hydroformylation; hydrogenation; ligand design; P ligands
资金
- Wuhan University [203273463, 203410100064]
- Ministry of Education of China
- National Natural Science Foundation of China [21372179, 21432007, 21502145]
Asymmetric hydroformylation represents one of the most efficient routes for the preparation of chiral aldehydes from alkenes in the presence of syngas in a perfect atom-economic way. During the past few decades, a variety of chiral ligands have been developed for the asymmetric hydroformylation. However, only a few ligands exhibit good performance in terms of the regio-and enantioselectivities. Additionally, for the chiral ligands developed up to now, only limited substrates were tolerated and no examples have led to the application of the asymmetric hydroformylation reaction on a commercial scale due to several technical challenges. This account provides a brief introduction of the current efficient chiral ligands for asymmetric hydroformylation and the ongoing efforts we have made in this field.
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