期刊
JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS
卷 140, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.jpcs.2020.109376
关键词
Bi2O4; Bi2O3; p-n junction; Photocatalysis
资金
- National Natural Science Foundation of China [21663012]
- Natural Science Foundation of Jiangxi Province [20181BAB203009]
- Scientific &Technological Project of Jiangxi Science and Technology Normal University [2015CXTD003]
Construction of p-n heterojunction is an effective strategy to obstacle the rapid recombination of photo-generated carriers for single photocatalyst. Herein, visible-light-active Bi2O3/Bi2O4 p-n junction was prepared by a one-pot hydrothermal method, using Bi(NO3)(3)center dot 5H(2)O, KCl, and NaBiO3 center dot 2H(2)O as precursors. The in-situ formed BiOCl reacts with NaBiO3.2H(2)O during the hydrothermal process, producing the target product of Bi2O3/Bi2O4 p-n heterojunction. As expected, the obtained Bi2O3/Bi2O4 heterojunction photocatalysts exhibited higher photocatalytic activity than Bi2O4 for the degradation of MO (methyl orange) and phenol under visible-light irradiation. The superior photocatalytic performance of Bi2O3/Bi2O4 hybrid is mainly attributed to the improved separation efficiency of e(-)-h(+) pair induced by the internal electric field of p-n junction. The present work may provide a rational and facile strategy to construct a highly efficient Bi2O4-based p-n heterojunction photocatalyst toward pollutant removal.
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