期刊
CHEMICAL COMMUNICATIONS
卷 52, 期 61, 页码 9538-9541出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc04597a
关键词
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资金
- NSF of China [21203022, 21261001, 21361001]
- Natural Science Foundation of Jiangxi Province of China [20143ACB20002, 20151BAB203001]
- Young Scientist Training Program of Jiangxi Province of China [20142BCB23018]
Herein, we demonstrate that Zn-MOF-74 enables the ultrafast and one-step generation of the Fe2O3@MOF composite once Zn-MOF-74 contacts with FeSO4 solution. This unique reaction can be further applied in catalysis of U(VI) reduction by Fe(II) under ambient conditions. The results provide a highly renovated strategy for U(VI) reduction by Fe(II) just under ambient conditions, which completely subvert all established methods about U(VI) reduction by Fe(II) in which O-2- and CO2-free conditions are absolutely required.
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