期刊
CHEMICAL COMMUNICATIONS
卷 52, 期 70, 页码 10636-10639出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc05329g
关键词
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资金
- National Natural Science Foundation of China [21472052]
- Science Foundation for Distinguished Young Scholars of Guangdong Province [2014A030306018 + 2015PT018]
- 1000 Youth Talents Plan
- Open Fund of the State Key Laboratory of Pulp and Paper Engineering of SCUT [201475]
- Foundation of Department of Education of Guangdong Province [2014KQNCX156]
A ruthenium-catalysed annulative transfer hydrogenation strategy, enabling straightforward access to tetrahydro fused-pyrazine derivatives from N-heteroaryl diamines and vicinal diols, has been demonstrated for the first time. Such a synthesis proceeds with unprecedented synthetic effectiveness including high step-and atom efficiency, generation of water as the sole by-product, short reaction time and no need for external high pressure H-2 gas, offering an important basis for the transformation of vicinal diols, a class of bio-mass derived resources, into functionalized products.
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