期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 388, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jhazmat.2019.121816
关键词
Tb-MOFs; VOCs; Sensor; Detection; Logic gate
资金
- Sichuan Science and Technology Program [2019YJ0525]
- Project of Education Department of Sichuan Province [18ZA0408]
- Opening Laboratory Project of Sichuan Normal University [KFSY2018022]
Volatile organic compounds (VOCs) are extremely harmful to the human body and environment, thus it is greatly meaningful and urgent to detect VOCs. In this work, terbium-based metal-organic frameworks (Tb-MOFs) have been prepared successfully via a facile and efficient route. These well-constructed Tb-MOFs architectures exhibit characteristic green emission of Tb3+ ion upon excitation of UV light. It is noteworthy that the Tb-MOFs can act as a convenient and efficient luminescent sensor for VOCs. Especially, the Tb-MOFs displayed high selectivity and superior sensitivity towards the sensing of styrene solution and vapor through fluorescence quenching mechanism. The Tb-MOFs can realize fast detection for styrene vapor with a response time of 30 s. The mechanism of fluorescence quenching of Tb-MOFs induced by styrene was also discussed. More importantly, we have designed a logic gate operation with the combination of the sensor for the intelligent detection of styrene. This developed type of lanthanide luminescent metal-organic frameworks (Ln-MOFs) based on the combination of fluorescence sensor and logic gate has a great application prospect in the detection of VOCs in daily life.
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