期刊
CHEMICAL COMMUNICATIONS
卷 52, 期 82, 页码 12206-12209出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc06190g
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资金
- Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-SC0001517]
- Fund for Scientific Research-Flanders [1510712N]
- University of Leuven [GOA/2011/03]
We report the first-order hyperpolarizabilities (bHRS values) of individualized, length-sorted (700 +/- 50 nm long) (6,5) SWNTs and corresponding polymer-wrapped (6,5) SWNT superstructures. These SWNT-based nano-hybrids feature semiconducting polymers that wrap the SWNT surface in an exclusive left-handed helical fashion. Manipulation of the polymer electronic structures in these well-defined nanoscale objects provides a new avenue to modulate the magnitude of bHRS at long wavelength (1280 nm).
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