期刊
CHEMICAL COMMUNICATIONS
卷 52, 期 18, 页码 3639-3642出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc10222g
关键词
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资金
- MINECO [MAT2013-45008-p, PCIN-2013-057]
- MINECO (Spain) [RyC-2012-11427]
- Royal Society (UK)
- Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [LDRD 7739, DE-AC0500OR22725]
- UT Battelle, LLC
The gate-opening phenomenon in ZIFs is of paramount importance to understand their behavior in industrial molecular separations. Here we show for the first time using in situ inelastic neutron scattering (INS) the swinging of the -CH3 groups and the imidazolate linkers in the prototypical ZIF-8 and ZIF-8@AC hybrid materials upon exposure to mild N-2 pressure.
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