期刊
JOURNAL OF ALLOYS AND COMPOUNDS
卷 821, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2019.153221
关键词
Perovskite solar cell; Simulation; Offset engineering; Efficiency
资金
- GCUF-Research Support Program [158-PHY-4]
- GCUF
In this paper a perovskite solar cell which consists of an inorganic hole transporting layer is studied using a SCAPS simulator. The primary structure of investigated solar cell is FTO/TiO2/MAPbI(3)/Spiro-OMeTAD/Ni which has PEC of 21.30%. The Cu2Zn(Sn1-x Ge-x)S-4 compound is good candidate as HTL in perovskite solar cells due to tunable band gap with different Ge/(Ge + Sn) ratios. The band gap was modulated from 1.5 for Cu2ZnSnS4 to 1.95 for Cu2ZnGeS4 with appropriate valence band offset engineering at the MAPbI(3)/Cu2Zn(Sn1-x Gex)S-4 interface. The solar cell performance was optimized by varying the Ge concentration, leading the PCE 20.86%. The data suggested that maximum efficiency is observed for Ge concentration x = 0.8. It is also observed that an appropriate VBO (0.20eV) with CZT(0.2)G(0.8)S hole transporting layer can be achieved. (C) 2019 Elsevier B.V. All rights reserved.
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