期刊
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
卷 2020, 期 31, 页码 4886-4892出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.202000610
关键词
Chalcogenation; Heterocycles; N-Oxides; Selenium; Transition-metal-free
资金
- Sookmyung Women's University Research grants [1-1503-0086]
Transition-metal-free and site-selective C-H selenylation of heterocyclic N-oxides with diselenides is described. This method can be also applied for the formation of C2-sulfenylated and C2-tellurinated quinoline derivatives. Notably, the simple reaction conditions with the use of anisole as a green solvent have been employed in this coupling reaction. Combined mechanistic investigations elucidate a plausible reaction mechanism of this process. The synthetic transformations demonstrate the utility of the developed method.
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