期刊
ENVIRONMENTAL SCIENCE & TECHNOLOGY
卷 54, 期 12, 页码 7107-7116出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.est.0c00740
关键词
-
资金
- Alfred P. Sloan Foundation [G-2017-9944, G-2016-7050, G-201911412, G-2019-12301]
It is important to improve our understanding of exposure to particulate matter (PM) in residences because of associated health risks. The HOMEChem campaign was conducted to investigate indoor chemistry in a manufactured test house during prescribed everyday activities, such as cooking, cleaning, and opening doors and windows. This paper focuses on measured size distributions of PM (0.001-20 mu m), along with estimated exposures and respiratory-tract deposition. Number concentrations were highest for sub-10 nm particles during cooking using a propane-fueled stovetop. During some cooking activities, calculated PM2.5 mass concentrations (assuming a density of 1 g cm(-3)) exceeded 250 mu g m(-3), and exposure during the postcooking decay phase exceeded that of the cooking period itself. The modeled PM respiratory deposition for an adult residing in the test house kitchen for 12 h varied from 7 mu g on a day with no indoor activities to 68 mu g during a simulated day (including breakfast, lunch, and dinner preparation interspersed by cleaning activities) and rose to 149 mu g during a simulated Thanksgiving day.
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