期刊
CHEMSUSCHEM
卷 13, 期 11, 页码 2935-2939出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.202000562
关键词
deuterium; water splitting; photocatalysis; quantum sieving; solar fuels
资金
- National Key R&D Program of China [2016YFA0602900, 2019YFC0408605]
- National Natural Science Foundation of China [21571064, U1701243]
- Research Project of Guangzhou Municipal Science and Technology Bureau [201903010035]
- Key-Area Research and Development Program of Guangdong Province [2019B110209002]
- Ministry of Education of the People's Republic of China Blue Project(Huizhou)
- Industry-Academic-Research Joint Invention Fund [CXZJHZ201735]
- Fundamental Research Funds for the Central Universities
- Key Laboratory of Fuel Cell Technology of Guangdong Province
Motivated by energy shortages and in view of current efforts to develop clean, renewable energy sources based on fusion, a solar-driven strategy has been developed for deuterium evolution. Deuterium is a critical resource for many aspects. However, the limited natural abundance of deuterium and the complexity of established technologies, such as quantum sieving (QS) for deuterium production under extreme conditions, pose challenges. The new method has the potential for robust and sustainable deuterium evolution, enabling deuterium production at a high rate of 9.745 mmol g(-1) h(-1). The activity, thermodynamic, and kinetic characteristics are also investigated and compared between photocatalytic heavy water (D2O) splitting and water (H2O) splitting. This study opens a new avenue to discover promising photocatalytic deuterium generation systems for advanced solar energy utilization and deuterium enrichment.
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