期刊
CHEMISTRY LETTERS
卷 49, 期 6, 页码 732-735出版社
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.200193
关键词
Iridium; C-H activation; Annulation
资金
- JSPS KAKENHI [JP19H02721]
Annulation of alpha,beta-unsaturated amides with electrondeficient 1,3-dienes gave 5,6-dihydropyridin-2(1H)-ones in the presence of a hydroxoiridium catalyst. The reaction proceeded via direct C-H alkylation of acrylamides with conjugated dienes, followed by intramolecular aza-Michael addition, thus giving dihydropyridinones stereoselectively in good yields.
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