期刊
CATALYSIS TODAY
卷 269, 期 -, 页码 82-87出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.cattod.2015.11.045
关键词
Ethanol; Butanol; Hydrotalcite; Mixed oxides; Guerbet
A highly versatile ethanol conversion process to selectively generate high value compounds is presented here. By changing the reaction temperature, ethanol can be selectively converted to >C-2 alcohols/oxygenates or phenolic compounds over hydrotalcite derived bi-functional MgO-Al2O3 catalyst via complex cascade mechanism. Reaction temperature plays a role in whether aldol condensation or the acetone formation is the path taken in changing the product composition. This article contains the catalytic activity comparison between the mono-functional and physical mixture counterpart to the hydrotalcite derived mixed oxides and the detailed discussion on the reaction mechanisms. (C) 2016 Published by Elsevier B.V.
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