4.4 Article

Radiolysis and and radionuclide production in a flowing-water target during fast 40Ca20+ irradiation

期刊

APPLIED RADIATION AND ISOTOPES
卷 158, 期 -, 页码 -

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.apradiso.2020.109049

关键词

Isotope harvesting; Isotope production; Ion exchange; Target corrosion; Radiolysis; G-value

资金

  1. U.S. Department of Energy, Office of Science, Office of Nuclear Physics, DOE Isotope Program [DOE-FOA-0001588]
  2. U.S. Department of Energy National Nuclear Security Administration Stewardship Science Graduate Fellowship [DE-NA0003864]
  3. Michigan State University

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A flowing-water target was irradiated with a 140 MeV/u, 8 nA 40Ca20+ beam to test the feasibility of isotope harvesting at the upcoming Facility for Rare Isotope Beams. Among other radionuclides, 2.6(2)E-6 48Cr and 5.6 (5)E-6 28 Mg nuclei were formed for every impingent 4OCa and were collected through ion exchange. Radiolysis-induced molecular hydrogen evolved from the target at an initial rate of 0.91(9) H2 molecules per 100 eV of beam energy deposited. No radiation-accelerated corrosion of the target material was observed.

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