期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 59, 期 36, 页码 15487-15491出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202005489
关键词
branched nickel; branching mechanisms; electrocatalysis; HMF oxidation; nanoparticle synthesis
资金
- Australian Research Council [LP150101014, FL150100060, DP190102659, DP200100143]
- UNSW Scientia Ph.D. Scholarship and Development Scheme
- Australian Research Council of Centre of Excellence in Convergent Bio-Nano Science and Technology [CE140100036]
- Microscopy Australia
- Mark Wainwright Analytical Centre and Electron Microscope Unit at the University of New South Wales
- Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany's Excellence Strategy [EXC 2033-390677874-RESOLV, FOR 2982 [433304666]]
- U.S. Department of Energy's NNSA [89233218CNA000001]
- U.S. Department of Energy's National Nuclear Security Administration [DE-NA-0003525]
- Projekt DEAL
- Australian Research Council [DP200100143] Funding Source: Australian Research Council
Controlling the formation of nanosized branched nanoparticles with high uniformity is one of the major challenges in synthesizing nanocatalysts with improved activity and stability. Using a cubic-core hexagonal-branch mechanism to form highly monodisperse branched nanoparticles, we vary the length of the nickel branches. Lengthening the nickel branches, with their high coverage of active facets, is shown to improve activity for electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF), as an example for biomass conversion.
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