期刊
NATURE CATALYSIS
卷 3, 期 3, 页码 225-244出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/s41929-019-0408-2
关键词
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资金
- Army Research Office MURI grant [W911NF1410263]
- National Science Foundation Center for Synthetic Organic Electrosynthesis [CHE-1740656]
Bioelectrocatalysis is a green, sustainable, efficient method to produce value-added chemicals, clean biofuels and degradable materials. As an alternative approach to modern biomanufacturing technology, bioelectrocatalysis fully combines the merits of both biocatalysis and electrocatalysis to realize the green, efficient production of target products from electricity. Here, we review the development status of bioelectrocatalysis, discussing the current challenges and looking toward future development directions. First, we detail the structure, function and modification methods of bioelectrocatalysis. Next, we describe the mechanism of electron transfer, including mediated electron transfer and directed electron transfer. Third, we discuss the impact of the electrode on bioelectrocatalysis. Then we analyse and summarize the application of bioelectrocatalysis methods in the production of chemicals, biofuels and materials. Finally, we detail future developments and perspectives on bioelectrocatalysis for electrosynthesis.
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