期刊
JOURNAL OF ENERGY CHEMISTRY
卷 40, 期 -, 页码 144-150出版社
ELSEVIER
DOI: 10.1016/j.jechem.2019.03.009
关键词
Asymmetric non-fullerene acceptors; Heteroatom substitution; Organic solar cells; Power conversion efficiency
资金
- National Natural Science Foundation of China (NSFC) [21674007, 21734001]
- National Research Foundation (NRF) of Korea [2012M3A6A7055540, 2015M1A2A2057506]
Research on asymmetric A-D-A structured non-fullerene acceptors has lagged far behind the development of symmetric counterpart. In this contribution, by simply replacing one sulfur atom in indacenodithiophene unit with a selenium atom, an asymmetric building block SePT and a corresponding asymmetric non-fullerene acceptor SePT-IN have been developed. Asymmetric SePT-IN achieved a high efficiency of 10.20% in organic solar cells when blended with PBT1-C, much higher than that of symmetric TPT-IN counterpart (8.91%). Our results demonstrated an effective heteroatom substitution strategy to develop asymmetric A-D-A structured non-fullerene acceptors. (C) 2019 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
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