期刊
CHEMPLUSCHEM
卷 85, 期 6, 页码 1095-1103出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cplu.201900737
关键词
fluorescence; mechanical properties; mechanochemistry; mechanophores; polymer chemistry
资金
- Freigeist-Fellowship of the Volkswagen Foundation
- European Commission (EUSMI) [731019]
In recent years, polymer mechanochemistry has evolved as a methodology to provide insights into the action-reaction relationships of polymers and polymer-based materials and composites in terms of macroscopic force application (stress) and subsequent deformation (strain) through a mechanophore-assisted coupling of mechanical and chemical phenomena. The perplexity of the process, however, from the viewpoint of mechanophore activation via a molecular-scaled disruption of the structure that yields a macroscopically detectable optical signal, renders this otherwise rapidly evolving field challenging. Motivated by this, we highlight here recent advancements of polymer mechanochemistry with particular focus on the establishment of methodologies for the efficient activation and quantification of mechanophores and anticipate to aptly pinpoint unresolved matters and limitations of the respective approaches, thus highlighting possible developments.
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