期刊
SCIENTIFIC REPORTS
卷 10, 期 1, 页码 -出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/s41598-020-58998-1
关键词
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资金
- Ministry of Education, Culture, Sports, Science, and Technology of Japan [17H03398, 17H05207]
- Tsinghua-Tohoku Collaborative Research Fund
- Grants-in-Aid for Scientific Research [17H05207, 17H03398] Funding Source: KAKEN
Mg2Sn is a potential thermoelectric (TE) material that can directly convert waste heat into electricity. In this study, Mg2Sn single-crystal ingots are prepared by melting under an Ar atmosphere. The prepared ingots contain Mg vacancies (V-Mg) as point defects, which results in the formation of two regions: an Mg2Sn single-crystal region without V-Mg (denoted as the single-crystal region) and a region containing V-Mg (denoted as the V-Mg region). The V-Mg region is embedded in the matrix of the single-crystal region. The interface between the V-Mg region and the single-crystal region is semi-coherent, which does not prevent electron carrier conduction but does increase phonon scattering. Furthermore, electron carrier concentration depends on the fraction of V-Mg, reflecting the acceptor characteristics of V-Mg. The maximum figure of merit zT(max) of 1.4(1) x 10(-2) is realised for the Mg2Sn single-crystal ingot by introducing V-Mg. These results demonstrate that the TE properties of Mg2Sn can be optimised via point-defect engineering.
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