期刊
ADVANCED ENERGY MATERIALS
卷 10, 期 11, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201903120
关键词
nanostructured catalysts; noble metals; structure engineering; water splitting
类别
资金
- Tencent Foundation
- Beijing Natural Science Foundation [JQ18005]
- National Basic Research Program of China [2017YFA0206701]
- National Natural Science Foundation of China [51671003]
- Peking University
- China Postdoctoral Science Foundation [2017M610022]
Electrochemical water splitting plays a crucial role in the development of clean and renewable energy production and conversion, which is a promising pathway to reduce social dependence on fossil fuels. Thus, highly active, cost-efficient, and robust catalysts must be developed to reduce the reaction overpotential and increase electrocatalytic efficiency. In this review, recent research efforts toward developing advanced electrocatalysts based on noble metals with outstanding performance for water splitting catalysis, which is mainly dependent on their structure engineering, are summarized. First, a simple description of the water-splitting mechanism and some promising structure engineering strategies are given, including heteroatom incorporation, strain engineering, interface/hybrid engineering, and single atomic construction. Then, the underlying relationship between noble metal electronic/geometric structure and performance for water splitting is discussed with the assistance of theoretical simulation. Finally, a personal perspective is provided in order to highlight the challenges and opportunities for developing novel electrocatalysts suitable for a wide range of commercial uses in water splitting for structural engineering applications.
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