期刊
NATURE COMMUNICATIONS
卷 11, 期 1, 页码 -出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/s41467-019-14194-y
关键词
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资金
- National Natural Science Foundation of China [51572286, 51772319, 51772320, 51972331]
- Natural Science Foundation of Jiangxi province [20181ACB20011]
- External Cooperation Program of the Chinese Academy of Sciences [121E32KYSB20190008]
- Six Talent Peaks Project of Jiangsu Province [XCL-170]
- Science and Technology Project of Nanchang [2017-SJSYS-008]
- Youth Innovation Promotion Association, CAS [2018356]
- Outstanding Youth Fund of Jiangxi Province [20192BCBL23027]
- Suzhou Industrial Science and Technology Program [SYG201737]
- National Key Research and Development Program of China [2019YFB2203402]
Intercalation-based inorganic materials that change their colours upon ion insertion/extraction lay an important foundation for existing electrochromic technology. However, using only such inorganic electrochromic materials, it is very difficult to achieve the utmost goal of full-colour tunability for future electrochromic technology mainly due to the absence of structural flexibility. Herein, we demonstrate an ultracompact asymmetric Fabry-Perot (F-P) nanocavity-type electrochromic device formed by using partially reflective metal tungsten as the current collector and reflector layer simultaneously; this approach enables fairly close matching of the reflections at both interfaces of the WO3 thin layer in device form, inducing a strong interference. Such an interference-enhanced device that is optically manipulated at the nanoscale displays various structural colours before coloration and, further, can change to other colours including blue, red, and yellow by changing the optical indexes (n, k) of the tungsten oxide layer through ion insertion.
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