期刊
ORGANIC LETTERS
卷 22, 期 5, 页码 1980-1984出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c00328
关键词
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资金
- National Natural Science Foundation of China [21772177, 21602202]
- Natural Science Foundation of Zhejiang Province [LY19B020016]
- Fundamental Research Funds of Zhejiang Sci-Tech University [2019Q065]
A palladium-catalyzed four-component carbonylative cyclization reaction for the expeditious construction of trifluoromethyl-containing trisubstituted imidazoles has been achieved. With readily accessible trifluoroacetimidoyl chlorides, propargyl amines, and diaryliodonium salts as the starting materials, the carbonylative transformation proceeds smoothly under mild conditions to enable the formation of multifunctionalized imidazole molecules in a one-pot, one-step manner. Diaryliodonium salts serve as both oxidants and aryl sources in the reaction.
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