期刊
ORGANIC LETTERS
卷 22, 期 4, 页码 1259-1264出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b04433
关键词
-
资金
- National Natural Science Foundation of China [21776171, 21636006, 21572122]
- Fundamental Research Funds for the Central Universities [GK201906005, GK201901001]
The aromatic aldehyde as a traceless directing group for the regionselective C-H alkylation catalyzed by rhodium(III) under aerobic atmospheric conditions has been developed. The process involves an aldehyde assisted direct addition of C-H bond to unsaturated electrophiles of acrylates or acrylic acids, and the subsequent decarbonylation. A trace amount of water is found to favor the reaction.
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