期刊
ORGANIC LETTERS
卷 22, 期 4, 页码 1326-1330出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.9b04645
关键词
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资金
- National Natural Science Foundation of China [21871240, 21672198]
- Fundamental Research Funds for the Central Universities [W1(2060190082)]
- State Key Program of National Natural Science Foundation of China [21432009]
A novel method of metal-free dehydrogenative silylation of enamides has been developed. The desired functionalized vinylsilane products were obtained in moderate to good yield and with high stereoselectivities. This protocol displays good tolerance of various functionalities. Furthermore, the high chemoselectivity of this reaction enables us to introduce different unsaturated C-C moieties to the products. The ease of further derivatization of the products to other useful compounds also demonstrates the highly synthetic utility of the current methodology.
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