期刊
MATERIALS RESEARCH BULLETIN
卷 121, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.materresbull.2019.110617
关键词
Black titania; Surface reduction; Anatase; Rutile; Ti-O bonds
资金
- National key research and development program [2016YFB0901600]
- NSF of China [61376056, 11404358]
- Science and Technology Commission of Shanghai [16JC1401700, 14520722000]
Though black titania has been widely investigated, the influence of crystal phase during the reduction process remains unknown. In the present study, we found that the rutile phase is preferentially reduced over anatase from detailed experimental investigations and a comprehensive understanding of selective breaking of Ti-O bonds in surfaced TiO6 octahedral motifs. This work may inspire an encouraging understanding in designing highly efficient black material for solar harvesting.
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