期刊
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN
卷 89, 期 2, 页码 161-173出版社
CHEMICAL SOC JAPAN
DOI: 10.1246/bcsj.20150307
关键词
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资金
- Japan Society for the Promotion of Science (JSPS) [24107002, 26840099]
- Japan Science and Technology Agency (JST), PRESTO
- Grants-in-Aid for Scientific Research [26840099, 24107002, 15H01063] Funding Source: KAKEN
Photosynthetically active chlorophyll molecules are biosynthesized from 5-aminolevulinic acid through protoporphyrin IX. The multistep enzymatic transformations were well investigated, but their pathways and reaction mechanisms have not been fully elucidated in the late stages. The biosynthetic pathways of (bacterio)chlorophylls from protoporphyrin IX are here described from a chemical viewpoint, especially focusing on the reduction processes of the C=C double to C-C single bonds. The regioselective and stereoselective trans-hydrogenation is performed in the enzymatic reductions.
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