期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 85, 期 4, 页码 2260-2265出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.9b02968
关键词
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资金
- Australian Research Council Future Fellowship [FT170100437]
- Australian Research Council [FT170100437] Funding Source: Australian Research Council
Singlet oxygen is a versatile reagent for the selective oxidation of organic compounds under mild reaction conditions. It is frequently invoked in biosynthetic pathways, so it is especially suitable for application in the biomimetic synthesis of natural products. Herein, we show that use of the singlet oxygen ene reaction, combined with [2 + 2] cycloadditions, leads to concise, divergent, and redox-economic total syntheses of several polycyclic members of the rhodonoid family of meroterpenoids.
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