期刊
JOURNAL OF INFRARED MILLIMETER AND TERAHERTZ WAVES
卷 41, 期 2, 页码 171-193出版社
SPRINGER
DOI: 10.1007/s10762-019-00651-8
关键词
THz-TDS; Optical basicity; Femtosecond laser modification; Refractive index
资金
- Kyocera Corporation
- Inamori School of Engineering
We studied femtosecond laser modifications of lanthanum aluminosilicate (SAL) glasses with 11-23 mol% La2O3 content. Refractive indices of these glasses were measured in the visible and terahertz frequencies and correlated to the change in the glass structure. The role of lanthanum provided a comparison to traditional glass modifiers within the glass network in terms of polarizability and optical basicity for femtosecond laser irradiation modification of the refractive index. Al-27 magic angle spinning nuclear magnetic resonance (MAS-NMR) was used to identify aluminum speciation within the SAL glasses. We used prism-coupling and terahertz time-domain spectroscopy (THz-TDS) for visible and THz refractive index measurements, respectively. Our results show a linear correlation between refractive index measurements in visible and terahertz frequencies with systematic rare-earth ion inclusions. In addition, our results demonstrate that THz-TDS can be utilized as a means of extending the detectable limits in refractive index measurements of disordered glass structures.
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