期刊
CHEMSUSCHEM
卷 13, 期 4, 页码 756-762出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201902889
关键词
charge separation efficiency; H-2 evolution; nanorods; photocatalysis; water splitting
资金
- Science and Technology Project of the Research Foundation of China Postdoctoral Science [2018M630982]
- Shenzhen Peacock Plan [827-000113]
- Educational Commission of Guangdong Province [2016KCXTD006]
- Science and Technology Project of Shenzhen [ZDSYS201707271014468]
- Guangdong Special Support Program
- Foundation for Distinguished Young Talents in Higher Education of Guangdong [2018KQNCX221]
Solar-driven H-2 evolution is an essential process for sustainable energy development. Currently, the greatest challenge is the development of efficient photocatalysts to drive this reaction, especially in pure water systems (without the use of a sacrificial agent). In this study, structural defects in Zn-Cd-S nanorod photocatalysts are found to increase charge separation efficiency significantly by sevenfold. Efficient H-2 evolution (352.7 mu mol h(-1) g(-1), 100 mg of catalyst) is achieved by using this defective Zn-Cd-S nanorod photocatalyst in the absence of sacrificial agents and precious metal cocatalysts under visible-light irradiation. Thus, this cocatalyst- and sacrificial-agent-free, visible-light-responsive system shows remarkable potential as a new artificial photosynthesis route for green H-2 production.
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