期刊
CHEMICAL GEOLOGY
卷 537, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.chemgeo.2020.119469
关键词
Mixing; Box models; Rayleigh; Reactive transport; Molecular scale simulations
资金
- DOE Office of Science SBR program [DE-SC0019198]
- DOE Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division, through Geosciences program at Lawerence Berkeley National Laboratory [DE-AC0205CH11231]
- U.S. Department of Energy (DOE) [DE-SC0019198] Funding Source: U.S. Department of Energy (DOE)
Though the utility of calcium isotopes is broad, examples of applications are still relatively sparse. Some of this paucity, as with many metal isotope systems, may derive from a perception that the analytical tool is difficult to access. Alternatively, potential users may be deterred by a sense that calcium isotopes are ambiguous, difficult to interpret, and/or complicated by too many interrelated processes. Here we provide an overview of the quantitative modeling approaches available to facilitate interpretation of calcium isotopes in Earth systems, in particular their ability to push interpretations beyond the qualitative. While no method is perfect, the variety of approaches described here offer an accessible toolset that is incredibly valuable. We suggest that the calcium isotope community should be expanding the use of such techniques, noting their limitations and striving to improve upon current methods over time.
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