期刊
BIORESOURCE TECHNOLOGY
卷 177, 期 -, 页码 8-16出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.biortech.2014.11.060
关键词
Diffusion; Dilute acid; Hydrolysis; Kinetic model; Lignocellulose
资金
- Program for New Century Excellent Talents in University [NCET-11-0477]
- Beijing Nova Program [Z131105000413056]
- Beijing Excellent Talents Cultivation Program [2013D009007000001]
- Beijing Higher Education Young Elite Teacher Project [YETP0317]
Kinetic experiments on the dilute sulfuric acid pretreatment of corn stover were performed. A high xylan removal and a low inhibitor concentration were achieved by acid pretreatment. A novel diffusion-hydrolysis coupled kinetic model was proposed. The contribution to the xylose yield was analyzed by the kinetic model. Compared with the inhibitor furfural negatively affecting xylose yield, the fast and slow-hydrolyzing xylan significantly contributed to the xylose yield, however, their dominant roles were dependent on reaction temperature and time. The impact of particle size and acid concentration on the xylose yield were also investigated. The diffusion process may significantly influence the hydrolysis of large particles. Increasing the acid concentration from 0.15 M to 0.30 M significantly improved the xylose yield, whereas the extent of improvement decreased to near-quantitative when further increasing acid loading. These findings shed some light on the mechanism for dilute sulfuric acid hydrolysis of corn stover. (C) 2014 Elsevier Ltd. All rights reserved.
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