期刊
CATALYSIS LETTERS
卷 150, 期 8, 页码 2377-2384出版社
SPRINGER
DOI: 10.1007/s10562-020-03141-y
关键词
Pd nanoparticles; Aminated activated carbon; Formic acid dehydrogenation
资金
- National Key R&D Program of China [2018YFB0604902]
Formic acid (FA) has attracted increasing interest in the utilization as a promising hydrogen carrier. Nitrogen-doped activated carbons were used as support to prepare well-dispersed Pd/C catalyst for hydrogen production from FA. The introduced N species adjusted the electronic properties of Pd and promoted dispersion of Pd, which were beneficial to improve the catalytic activity. Pd supported on the activated carbon aminated at 950 degrees C (the particle size of Pd is 2.8 +/- 0.1 nm) showed the highest turnover frequency (TOF) of 1631 h(-1) at 30 degrees C.
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