期刊
APPLIED SURFACE SCIENCE
卷 515, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.apsusc.2020.146003
关键词
Magnetically assembled electrode; Chlorine evolution; Oxygen evolution; Lead oxide; Tin dioxide; 2.5D electrode
类别
资金
- National Natural Science Foundation of China [21706153]
- Natural Science Basic Research Plan in Shaanxi Province of China [2018JQ2066]
The variable composition in wastewater makes the electrochemical oxidation (EO) treatment method difficult to maintain its full-time high efficiency. In this study, the Cl- concentration was investigated as the first key variable factor. A magnetically assembled electrode (MAE) architecture with flexibility and variability was utilized to treat such variable organic wastewater. The main electrode of MAE, i.e., Ti/Pb3O4 anode offered the MAE with the high chlorine evolution ability and stability at high NaCl concentration, while the auxiliary electrodes of MAE, i.e., Sb-SnO2 coated magnetic particles (Fe3O4/Sb-SnO2), provided the MAE with sufficient EO ability at low NaCl concentration. The degradation experiments on azo dye and phenol using MAE with different loading amount of Fe3O4/Sb-SnO2 were carried out. The results provided a design rule in adjusting the optimized modular components for achieving higher EO efficiency under different Cl(- )concentrations. The relationships between MAE's surface composition/structure, electrochemical properties, degradation efficiency and Cl(- )concentration were further revealed. Finally, the operating mechanism of the MAE was discussed and verified.
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