期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 59, 期 8, 页码 3322-3328出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201912756
关键词
amorphous materials; photoluminescence; photothermal conversion; supercritical CO2; VS2 nanosheets
资金
- National Natural Science Foundation of China [51173170, 21571157, 21703207, 21773216]
- China Postdoctoral Science Foundation [2018T110738]
In two-dimensional (2D) amorphous nanosheets, the electron-phonon coupling triggered by localization of the electronic state as well as multiple-scattering feature make it exhibit excellent performance in optical science. VS2 nanosheets, especially single-layer nanosheets with controllable electronic structure and intrinsic optical properties, have rarely been reported owing to the limited preparation methods. Now, a controllable and feasible switching method is used to fabricate 2D amorphous VS2 and partial crystallized 2D VO2(D) nanosheets by altering the pressure and temperature of supercritical CO2 precisely. Thanks to the strong carrier localization and the quantum confinement, the unique 2D amorphous structures exhibit full band absorption, strong photoluminescence, and outstanding photothermal conversion efficiency.
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