期刊
ACS APPLIED MATERIALS & INTERFACES
卷 12, 期 13, 页码 15928-15933出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.0c01173
关键词
all-inorganic perovskite; interfacial modification; light-emitting thermal evaporation; charge transport
资金
- State Key Laboratory of Luminescence and Applications [SKLA-2019-07]
- Natural Science Foundation of Hebei Province [F2019202252, F2019202294]
- National Natural Science Foundation of China [61774154, 51672068, 51902082]
- Jilin Province Science and Technology Research Project [20180201029GX]
- Natural Science Foundation of Tianjin [17JCYBJC41500]
Efficient inorganic perovskite light-emitting devices (PeLEDs) with a vacuum-deposited CsPbBr3 emission layer were realized by introducing an ultrathin 2-phenylethanamine bromide interlayer. The PEA(+) cations not only passivated the nonradiative defects by terminating on the CsPbBr3 surface but also regulated the charge transport to balance the hole and electron transport. Consequently, the PeLEDs exhibit significantly promoted performance with a turn-on voltage of 3 V, a maximum current efficiency of 14.64 cd A(-1), and an external quantum efficiency of 4.10%. Our work would provide instructive guidance for realizing efficient PeLEDs based on a vacuum processing method via focusing on the interface modification between the perovskite layer and the carrier transport layer.
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