期刊
ACS APPLIED MATERIALS & INTERFACES
卷 12, 期 7, 页码 8704-8712出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.9b21048
关键词
carbon nanotube; polyimide; electromagnetic interference shielding; heat resistance
资金
- National Natural Science Foundation of China [21704070, 51673134, 51721091]
- Programme of Introducing Talents of Discipline to Universities [B13040]
- Fundamental Research Funds for the Central Universities [2017SCU04A03, sklpme2017306, 2012017yjsy102]
Excellent electromagnetic interference (EMI) shielding ability, light weight, and good heat resistance are highly required for practical applications of EMI shielding materials, such as in areas of aerospace, aircraft, and automobiles. Herein, a lightweight and robust carbon nanotube (CNT)/polyimide (PI) foam was developed for efficient and heat-resistant EMI shielding. Thanks to poly(vinyl pyrrolidone) (PVP) as a surfactant that not only promotes the uniform dispersion of CNTs to form perfect CNT conductive networks but also can be removed in situ during the polymerization process, the density of resultant CNT/PI foam is only 32.1 mg.cm(-3), and the EMI shielding effectiveness (EMI SE) is up to 41.1 dB, which represents one of the highest EMI SE values compared to previously reported polymer-based foams. The CNT/PI foam also achieves the absorption coefficient (A) of up to 82.3%, which is very impressive in CNT/polymer foams at comparable EMI SE levels. The PI matrix endows the foam with excellent heat resistance. The as-prepared CNT/PI foam presents a higher EMI SE than 35 dB even after being subjected to the flame of an alcohol burner. Moreover, the compressive strength and compressive modulus are up to 240.9 and 323.9 kPa. These results indicate its certain application potential in the harsh requirement of aeronautics and aerospace industries as a highly efficient and lightweight EMI shielding material.
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