期刊
ACS APPLIED MATERIALS & INTERFACES
卷 12, 期 1, 页码 1850-1857出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsami.9b17052
关键词
superhydrophobic; superoleophilic; metal mesh; phytic acid; anticorrosion; environmentally friendly; oil spill cleanup
资金
- National Natural Science Foundation of China [51703235, 51973231, U1809213, U1809214]
Phytic acid (PA), which is a natural and innoxious plant constituent, can strongly adsorb on the metal surface because of its six phosphate groups. In this work, based on the chelating properties of PA and the reaction between PA and hydrolyzable vinyltriethoxysilane (VTES), we developed a novel and facial strategy to generate hierarchical-layer nanospheres on the metal mesh surface and fabricated robust superhydrophobic and superoleophilic miniature metal mesh ships. Because of their superwetting properties, the modified meshes could easily remove and recycle the oil spills from the water surface (>90% collection efficiency), and have high oil/water separation capacity (>96%). The excellent stability, corrosion resistance, and robust mechanical durability endow the modified mesh ships with more advantages in a marine environment. We envision that these superhydrophobic meshes modified with PA and VTES are sustainable, environmentally friendly, and easy to scale up and hence display great potential in practical application.
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