期刊
CHEMELECTROCHEM
卷 6, 期 20, 页码 5331-5339出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/celc.201901493
关键词
Mn2Sb2O7; reduced graphene oxide; lithium-ion batteries; high capacity; cyclic stability
For the advancement of lithium-ion batteries (LIBs), metal oxides with high theoretical specific capacities have been explored as anodes. Herein, we report a new metal oxide, Mn2Sb2O7-anchored reduced graphene oxide (Mn2Sb2O7/RGO), as an advanced anode for LIBs. The Mn2Sb2O7/RGO anode exhibits a higher capacity and better capacity retention compared to Mn2Sb2O7, because the close contact between Mn2Sb2O7 and RGO facilitates charge transfer during cycling. The discharge capacity of Mn2Sb2O7/RGO reaches 706.72 mAh g(-1) at 200 mA g(-1) after 200 cycles. Even at 1000 mA g(-1), the capacity loss per cycle of Mn2Sb2O7/RGO is only 0.0344 % for 600 cycles, indicating an excellent high-rate cyclic stability compared to other Sb-based oxides. These results forecast that Mn2Sb2O7/RGO is a potential anode for LIBs, providing a new insight into the selection of high-performance anodes.
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