期刊
JOURNAL OF POWER SOURCES
卷 440, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jpowsour.2019.227113
关键词
Low cobalt; NMC; Layered oxides; Lithium-ion; Li/Ni exchange; X-ray absorption
资金
- U.S. DOE [DE-AC02-06CH11357]
- Vehicle Technologies Office (VTO), Hybrid Electric Systems Program, David Howell, Battery R&D, Peter Faguy, at the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy
- Canadian Light Source
The necessity of developing low-cobalt cathode oxides for lithium-ion batteries is increasingly apparent. The most popular strategy followed thus far in addressing this issue has been the development of LiNiO2-like, Ni-rich, layered LiMO2 (M = Ni, Mn, Co; NMC) oxides with low Mn and Co contents, e.g., NMC-811. However, safety, cycle-life, and even cost could remain critical barriers to the success of such cathode materials. Herein an alternative to LiNiO2-based, low-cobalt cathodes is suggested based on modifications to the prototypical cobalt-free, layered oxide, LiNi0.5Mn0.5O2.
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