期刊
JOURNAL OF LUMINESCENCE
卷 214, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jlumin.2019.116545
关键词
Ce,Mg:LuYAG ceramics; Y admixture; Scintillation yield; Decay kinetics
类别
资金
- National Natural Science Foundation of China, China [61775226, 61675221]
- National key R&D Program of China [2017YFB0310500, 2016YFB0701004]
- Czech Science Foundation [16-15569S]
- Ministry of Education, Youth and Sports of Czech Republic [LO1409, CZ. 02.1.01/0.0/0.0/16_013/0001406]
- ASCR-CAS bilateral mobility project
Ce,Mg:LuYAG transparent ceramics were successfully fabricated by the solid state reaction method. The results of x-ray diffraction, photoluminescence, light yield, scintillation decay and thermoluminescence are analyzed to provide better understanding of the influence of the Y3+ admixture in LuAG on the lattice structure, electronic band structure, energy-level structure of Ce3+ centers and scintillation properties. The lattice parameter of Ce,Mg:LuYAG ceramics shows a linear growth with the increasing Y content, which is in agreement with Vegard's law. Reducing the Lu-to-Y ratio in the LuYAG matrix, the Ce3+ 5d(1) energy level shifts to a lower energy, the forbidden gap becomes narrower and the electron traps become shallower. Furthermore, the increase of light yield and accelerated slow scintillation component are found with increasing Y admixture. After optimization, the light yield of Ce,Mg:Lu0.5Y2.5Al5O12 ceramics is achieved to 24,500 ph/MeV with 1 mu s shaping time, which is 40% higher than the value in the Y-free Ce,Mg:LuAG ceramic sample.
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