期刊
JOURNAL OF ALLOYS AND COMPOUNDS
卷 817, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2019.152695
关键词
SrTiO3; Energy storage; Dielectric breakdown strength; Charge-discharge performance
资金
- National Natural Science Foundation of China [51872175]
- International Cooperation Projects of Shaanxi Province [2018KW-027]
Ca0.5Sr0.5(TaxTi1-1.25x)O-3-2 wt%SiO2 ceramic samples were fabricated by solid state method. XRD data showed all samples are assigned to perovskite structure, dense microstructure and relatively large grain size were displayed by SEM. Moreover, the effect of Ta5+ ion doping on increased resistivity and energy barrier height were analysed by impendance spectra. Exceptional energy storage performances which are 2 J/cm(3) in energy density and 96% in energy efficiency under breakdown strength of 360 kV/cm can be obtained in the sample with x = 0.024, also possessing over 80% efficiency in a wide range of temperature (20-120 degrees C). Additionally, pulsed charging and discharging tests were carried out aiming to evaluate the practical performance of ceramic materials. The prominent parameters I-max of 32.2 A, C-D of 256.1 A/cm(2), P-D of 15.4 MW/cm(3) and outstanding temperature stability (20-120 degrees C) were achieved in the sample with x= 0.024 as well, releasing stored energy sharply (t(0.9) < 25 ns). These properties verified this lead-free linear dielectric ceramic can be promising candidate for wider applications in the fields of energy-storage and charge-discharge. (C) 2019 Elsevier B.V. All rights reserved.
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