期刊
DYES AND PIGMENTS
卷 170, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.dyepig.2019.107630
关键词
Perovskite solar cell; Graphene; APTES; Graphene quantum dot; PCBM; Transparent conductive electrode; Flexible
资金
- National Research Foundation of Korea - Ministry of Science, ICT and Future Planning [NRF-2017R1A2B3006054]
In recent years, organic-inorganic hybrid perovskite solar cells (PSCs) have received strong attention due to their high power conversion efficiency (PCE) and low cost. Here, we first employ 3-aminopropyl triethoxysilane (APTES)-treated graphene (GR) as a transparent conductive electrode (TCE) and quantum dots (GQDs)-doped phenyl C61 butyric acid methyl ester (PCBM) as an electron transport layer (ETL) for flexible PSCs. By increasing the concentration of GQDs to 2.5 mg/L, the PCE of the PSCs with GR/APTES TCE increases up to 16.4 and 15.0% on rigid and flexible substrates, respectively due to the reduced charge recombination at the ETL/perovskite interface and improved conductivity of the ETL. The flexible PSCs exhibit excellent bending stability by maintaining similar to 80% of the original PCE even after 3000 bending cycles at a curvature radius of 4 mm, resulting from the improved flexibility by the APTES interlayer.
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