4.7 Article

A simple and universal strategy to deposit Ag/polypyrrole on various substrates for enhanced interfacial solar evaporation and antibacterial activity

期刊

CHEMICAL ENGINEERING JOURNAL
卷 384, 期 -, 页码 -

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2019.123379

关键词

Solar distillation; Photothermal material; Interfacial water evaporation; Anti-biocorrosion

资金

  1. National Natural Science Foundation of China [51873047, 51761145031]
  2. State Key Laboratory of Urban Water Resource and Environment in HIT of China [2019DX10]
  3. Scientific Research Foundation for Returned Scholars of Heilongjiang Prov [LC2017023]

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Solar-driven distillation is now considered as a rising technology for the supply of fresh water in the rare areas. As the crucial part of solar distillation, photothermal materials have been flourished investigated. Herein, we report a universal and facile method to construct a photothermal layer on various substrates to enhance the interfacial water evaporation via polypyrrole (PPy) polymerization and silver nanoparticles (Ag NPs) deposition. The photothermal Ag/PPy layer was firmly coated on six different substrates with an average solar absorption of 95.4% and Ag loading of 94.3 mg/L. One of the optimized resultant membranes (substrate is cellulose fibers) presents the ultrahigh solar evaporation rate of 1.55 kg m(-2)h(-1) and a corresponding light-to-vapor efficiency of 92.6% with a silver loading of 74 mu g cm(-2). Bacterial diffusion inhibition zone experiments revealed clear antibacterial effects of the Ag/PPy membrane on bacteria. Furthermore, the Ag NPs deposited membrane had a rechargeability for multiple times upon their depletion, indicating sustainable anti-bacteria potential. Hence, our facial fabricated photothermal Ag/PPy layer can apply to substrates with different types for enhanced photothermal and anti-biocorrosion capacity, and may pave a new way to the long-term practical sustainable technique for the clean water production application.

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