期刊
CARBOHYDRATE POLYMERS
卷 230, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.carbpol.2019.115642
关键词
Wastewaterremediation; 3D hybridhydrogel; Multifunction; Photocatalyticdegradation; water/oil separation; Antibacterial
资金
- National Natural Science Foundation of China [31700510]
- Natural Science Foundation of Shaanxi Province [2018JQ3013]
- Key Scientific Project of Sichuan Educational Department [18ZA0315]
- High-level Foreign Experts Project [GDT20186100425]
3D Hydrogel is one of the most popular adsorbents for water remediation due to its excellent concentration/adsorption capacity. However, it remains a challenge to use the hydrogel alone for treating complex wastewater. In this work, we designed and fabricated a versatile bio-based hybrid hydrogel consisting of Ag NPs@ MIL-100(Fe) photocatalysts and guargum (GG) via facile blending and self-crosslinking. The hybrid hydrogel integrated with multifunctions of dye adsorption and degradation, oil/water separation and antibacterial properties, thus enabling its applications in complex wastewater remediation process. The presence of Ag nanoparticles (Ag NPs) not only enhanced the photocatalytic activity of MIL-100(Fe), but also imparted the antibacterial activity of Ag NPs@MIL-100(Fe)/ GG hydrogel. Particularly, the bio-based GG hydrogel scaffold showed excellent injectable, remodeling, and self-healing properties, which enabled an effective oil/water separation ability (silicone oil, cyclohexane and canola oil) and facilitated the recyclability/sustainability of the nano-photocatalyst powders. This novel multifunctional 3D hybrid hydrogel provides new opportunities for wastewater remediation purpose.
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