4.4 Article

A solid support generator of the Auger electron emitter rhodium-103m from [103Pd]palladium

期刊

APPLIED RADIATION AND ISOTOPES
卷 156, 期 -, 页码 -

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.apradiso.2019.108985

关键词

Auger radiotherapy; Radionuclide generator; Rhodium-103m; Palladium-103; 16aneS4

资金

  1. Independent Research Fund Denmark [DFF-6111-003921]

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Auger electron therapy is an attractive modality for targeting microscopic tumors. Rhodium-103 m (Rh-103m, T-1/2 = 56.1 min) is a promising Auger electron emitter that can be obtained as the decay product of palladium-103 (Pd-103, T-1/2 = 16.99 days). Pd-103 was chelated in a lipophilic derivative of the 16aneS4 macrocycle and the complex was trapped on a C18 cartridge. Elution with dilute hydrochloric acid gave radiochemically pure Rh-103m. We hypothesize this to be through a combination of the Szilard-Chalmers effect and transient ionization.

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