期刊
ADVANCED FUNCTIONAL MATERIALS
卷 30, 期 5, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201907150
关键词
bottom contacts; charge carrier mobility; floating-catalyst chemical vapor deposition; nanomaterials; ultraclean carbon nanotube devices
类别
资金
- DFG/ATUMS (Alberta/TU Munchen Graduate School Functional Hybrid Materials) [IRTG 2022]
- European Union Seventh Framework Program FP7 Nanosciences, Nanotechnologies, Materials and new Production Technologies (FP7/2007-2013) [604472]
- Aalto (university) Energy Efficiency (AEF) Research Program through the MOPPI project
- Academy of Finland (Luonnontieteiden ja Tekniikan Tutkimuksen Toimikunta) [286546, 292600]
- TEKES Finland [3303/31/2015, 1882/31/2016]
In this work, a fast approach for the fabrication of hundreds of ultraclean field-effect transistors (FETs) is introduced, using single-walled carbon nanotubes (SWCNTs). The synthesis of the nanomaterial is performed by floating-catalyst chemical vapor deposition, which is employed to fabricate high-performance thin-film transistors. Combined with palladium metal bottom contacts, the transport properties of individual SWCNTs are directly unveiled. The resulting SWCNT-based FETs exhibit a mean field-effect mobility, which is 3.3 times higher than that of high-quality solution-processed CNTs. This demonstrates that the hereby used SWCNTs are superior to comparable materials in terms of their transport properties. In particular, the on-off current ratios reach over 30 million. Thus, this method enables a fast, detailed, and reliable characterization of intrinsic properties of nanomaterials. The obtained ultraclean SWCNT-based FETs shed light on further study of contamination-free SWCNTs on various metal contacts and substrates.
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